Cannot upload more than 60GB on S3 through UI or console access

The limit for uploads via the Console is 160GB, anything bigger use the command line

• Upload an object in a single operation by using the AWS SDKs, REST API, or AWS CLI – With a single PUT operation, you can upload a single object up to 5 GB in size.
• Upload a single object by using the Amazon S3 console – With the Amazon S3 console, you can upload a single object up to 160 GB in size.
• Upload an object in parts by using the AWS SDKs, REST API, or AWS CLI – Using the multipart upload API operation, you can upload a single large object, up to 5 TB in size.

https://docs.aws.amazon.com/AmazonS3/latest/userguide/upload-objects.html